| CPC H01L 21/02312 (2013.01) [H01L 21/764 (2013.01)] | 17 Claims |

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1. A substrate processing method comprising:
forming a protective layer on a pattern structure including an upper surface, a lower surface, and a side surface connecting the upper surface and the lower surface;
supplying a fluorine-containing gas under a first plasma condition comprising a first frequency and first process pressure to form fluorine-terminated sites on the protective layer;
purging the fluorine-containing gas;
supplying a hydrogen-containing gas under a second plasma condition comprising a second frequency higher than the first frequency and second process pressure higher than the first process pressure to form hydrogen-terminated sites on the protective layer;
purging the hydrogen-containing gas;
supplying a silicon-containing source gas to form Si—H-terminated sites, wherein the forming of the Si—H-terminated sites is promoted on the hydrogen-terminated sites and inhibited on the fluorine-terminated sites;
purging the silicon-containing source gas;
forming an interlayer insulating layer on the protective layer by supplying a reactive gas having reactivity with the Si—H-terminated sites; and
purging the reactive gas.
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