| CPC H01L 21/0228 (2013.01) [C23C 16/45527 (2013.01); H01L 21/02211 (2013.01); H01L 21/0254 (2013.01); H01L 21/28194 (2013.01); C23C 16/34 (2013.01)] | 19 Claims |

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1. A method of forming a thin film comprising titanium nitride (TiN), the method comprising:
providing a semiconductor substrate comprising a non-metallic surface;
forming on the non-metallic surface a seed layer comprising a TiSiN layer by thermal atomic layer deposition (ALD) without aid of a plasma; and
forming on the seed layer and in situ in a same chamber a TiN layer by thermal ALD without aid of a plasma,
wherein forming the seed layer comprises alternatingly exposing the semiconductor substrate to one or more cycles, each of the one or more cycles comprising an exposure to a Si precursor, an exposure to a Ti precursor following the exposure to the Si precursor without an intervening exposure to a N precursor, and an exposure to a N precursor following the exposure to the Ti precursor without an intervening exposure to a Si precursor, thereby forming the TiSiN layer,
wherein the seed layer is distinct from the TiN layer and has a thickness of about 0.5 nm to about 5 nm, and
wherein a thickness ratio of the TiN layer to the seed layer exceeds 5.
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