| CPC G02B 1/002 (2013.01) | 2 Claims |

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1. An effective nonlinear optical coefficient optimization method for langasite group solid solution crystals, wherein the langasite group crystal A3BC3D2O14 mainly comprises langanite (LGN) crystal, langatate (LGT) crystal and langasite (LGS) crystal; the solid solution crystals are formed by adjusting a component proportion of langasite group crystals with the same structure, so that different ions mix and occupy sites in a polyhedral group, and a polyhedral lattice structure, distortion degree, refractive index and refractive dispersion of the solid solution crystal are changed,
wherein the B-site group is mixed with and occupied by Ga3+, Nb5+, Ta5+, Ti4+, Zr4+, Hf4+, Sn4+, and Sb5+ ions;
the D-site group is mixed with and occupied by Ga3+, Ge4+, Si4+ ions; or
different ions mix and occupy sites in two types of polyhedral groups of B-site and D-site at same time; Ga3+ and Zr4+ ions mix and occupy sites at the B-site, and Ga3+ and Si4+ ions mix and occupy sites at the D-site to form lanthanum gallium zirconate solid solution crystals.
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