| CPC H01L 21/4846 (2013.01) [C25D 3/38 (2013.01); C25D 5/022 (2013.01); C25D 5/08 (2013.01); C25D 5/18 (2013.01); C25D 5/48 (2013.01); C25D 5/605 (2020.08); C25D 5/617 (2020.08); C25D 7/123 (2013.01); C25D 17/001 (2013.01); C25D 21/12 (2013.01); C25F 3/02 (2013.01); C25F 3/22 (2013.01); H01L 24/11 (2013.01); H01L 24/13 (2013.01); H01L 24/742 (2013.01); H01L 24/81 (2013.01); H01L 2224/11462 (2013.01); H01L 2224/11831 (2013.01); H01L 2224/11901 (2013.01); H01L 2224/13078 (2013.01); H01L 2224/1308 (2013.01); H01L 2224/13147 (2013.01); H01L 2224/81895 (2013.01)] | 25 Claims |

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1. A method of preparing copper features for direct copper-copper bonding, the method comprising:
forming a plurality of first copper features on a first substrate, each of the plurality of first copper features having nanotwinned copper structures; and
electroplanarizing the plurality of first copper features by anodically biasing the first substrate, contacting the plurality of first copper features with an electrolyte, and electrochemically removing a portion of exposed copper from the first copper features prior to directly bonding the first substrate to a second substrate having a plurality of second copper features disposed on the second substrate, wherein electroplanarizing the plurality of first copper features comprises:
electroetching copper of the plurality of first copper features below a critical potential; and
electropolishing the copper of the plurality of first copper features above the critical potential.
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