| CPC C23C 16/45525 (2013.01) [C23C 16/401 (2013.01); H01L 21/02164 (2013.01); H01L 21/0228 (2013.01)] | 14 Claims |

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1. A method of filling a gap formed on a substrate, the method comprising:
forming a first reaction inhibition layer on a side wall of the gap;
forming a first precursor layer by adsorbing a first reactant into a bottom of the gap and into the side wall of the gap around the bottom of the gap; and
forming a first atomic layer on the bottom of the gap and the side wall of the gap around the bottom of the gap by adsorbing a second reactant into the first precursor layer,
wherein the forming of the first reaction inhibition layer comprises,
adsorbing a first reaction inhibitor into the side wall of the gap, and
forming a second reaction inhibitor by removing a specific ligand from the first reaction inhibitor,
wherein the first reaction inhibitor is adsorbed to have a density gradient in which a density of the first reaction inhibitor decreases toward the bottom of the gap, and
the second reaction inhibitor comprises a precursor material that does not react with the second reactant.
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