CPC C30B 29/42 (2013.01) [C30B 11/002 (2013.01); C30B 11/006 (2013.01); H01L 29/20 (2013.01); H01L 29/32 (2013.01); H01L 29/36 (2013.01); H01L 29/30 (2013.01); H01S 5/3013 (2013.01)] | 20 Claims |
1. A method for forming single crystal gallium arsenide substrates, the method comprising:
sealing charge material comprising polycrystalline gallium arsenide, a gallium arsenide seed crystal, B2O3 encapsulant, and carbon in a crucible;
sealing the crucible in a quartz ampoule;
performing a vertical gradient freeze crystal growth process by heating the ampoule using a multi-zone heating system to progressively melt the charge material until a portion of the seed crystal is melted;
starting growth from the partially melted seed by implementing a controlled cooling of the multi-zone heating system at a rate of 0.1 to 2 degree C./hour;
applying a temperature gradient of between 0.2 to 5 C/cm at a melt-crystal interface; and
maintaining a ratio of 1.0 to 4 between a temperature gradient above the melt-crystal interface to a temperature gradient below the melt-crystal interface in the multi-zone heating system to form a solidified gallium arsenide crystal.
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