| CPC G01N 1/36 (2013.01) [G01N 1/28 (2013.01); G01N 1/286 (2013.01); G01N 2001/2873 (2013.01)] | 34 Claims |

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1. A method for iteratively enlarging a sample of interest comprising biomolecules for microscopy, the method comprising the steps of:
a) contacting the sample with a biomolecule anchoring agent (BAA), wherein the BAA comprises a biomolecule binding moiety and an anchor;
b) embedding the sample in a first swellable material, wherein the biomolecules in the sample anchor to the first swellable material;
c) subjecting the sample to a disruption of the endogenous physical structure of the sample;
d) swelling the first swellable material resulting in an enlargement of the sample;
e) re-embedding the enlarged sample in a non-swellable material to form an enlarged sample hybrid;
f) embedding the enlarged sample hybrid in a second swellable material, wherein the second swellable material is the same as the first swellable material; and
g) swelling the second swellable material to further enlarge the sample,
wherein the biomolecules in the sample remain anchored to the first swellable material.
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