| CPC A61L 27/227 (2013.01) [A61L 27/3604 (2013.01); A61L 27/52 (2013.01)] | 20 Claims |

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1. A composition comprising tyramine-substituted silk fibroin, wherein a first phenol group of the tyramine-substituted silk fibroin is covalently crosslinked to a second phenol group of the tyramine-substituted silk fibroin.
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