| CPC H01M 4/366 (2013.01) [H01M 4/13 (2013.01); H01M 4/38 (2013.01); H01M 4/62 (2013.01); H01M 4/664 (2013.01); H01M 10/0525 (2013.01); H01M 2004/021 (2013.01)] | 18 Claims |

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1. An anode for an energy storage device comprising:
a current collector;
a first lithium storage layer overlaying the current collector;
a first intermediate layer overlaying at least a portion of the first lithium storage layer; and
a second lithium storage layer overlaying the first intermediate layer,
wherein the first lithium storage layer is a continuous porous lithium storage layer comprising a total content of silicon, germanium, or a combination thereof, of at least 40 atomic %,
and wherein the first intermediate layer comprises a first sublayer in contact with an underlying lithium storage layer and a second sublayer overlaying the first sublayer and in contact with an overlying lithium storage layer, the first sublayer having different a chemical composition than the second sublayer.
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