| CPC C23C 16/02 (2013.01) [C23C 16/4402 (2013.01); C23C 16/45557 (2013.01); C23C 16/45553 (2013.01)] | 16 Claims |

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1. A method, comprising:
delivering vanadium tetrachloride from a bulk supply tank to a delivery vessel as a gas;
after delivering vanadium tetrachloride to the delivery vessel, adding excess chlorine gas to the delivery vessel, thereby mitigating the decomposition of vanadium tetrachloride into decomposition products of the vanadium tetrachloride;
periodically delivering the vanadium tetrachloride from the delivery vessel to a reaction chamber configured for depositing a material and in fluid communication with the delivery vessel; and
sequentially applying the vanadium tetrachloride and a reactant to a substrate disposed in the reaction chamber to form a layer comprising vanadium on the substrate by a cyclical deposition process.
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