| CPC H01J 37/32449 (2013.01) [C23C 16/0272 (2013.01); C23C 16/345 (2013.01); C23C 16/40 (2013.01); C23C 16/403 (2013.01); C23C 16/4408 (2013.01); C23C 16/45536 (2013.01); C23C 16/4554 (2013.01); C23C 16/45553 (2013.01); C23C 16/45555 (2013.01); C23C 16/50 (2013.01); C23C 16/54 (2013.01); H01J 37/32743 (2013.01); H01J 37/32752 (2013.01); H01J 2237/20278 (2013.01); H01J 2237/332 (2013.01); H01J 2237/3321 (2013.01)] | 12 Claims |

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1. A method of forming a coating of material on a substrate, the method comprising:
forming a plasma of a first precursor and an oxygen-containing precursor, wherein the first precursor and the oxygen-containing precursor are provided in a first flow rate ratio;
depositing a first layer of material on the substrate, wherein the first layer of material is characterized by a first concentration of hydrogen;
while maintaining the plasma, adjusting the first flow rate ratio to a second flow rate ratio; and
depositing a second layer of material on the first layer of material, wherein the second layer of material is characterized by a second concentration of hydrogen less than the first concentration of hydrogen, and wherein a flow-rate ratio of the oxygen-containing precursor to the first precursor is maintained at greater than or about 2.0:1 while depositing the first layer of material on the substrate, depositing the second layer of material on the first layer of material, or both.
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