| CPC D01F 4/02 (2013.01) [C08L 89/00 (2013.01); B82Y 40/00 (2013.01); D10B 2211/04 (2013.01); D10B 2211/22 (2013.01)] | 16 Claims |

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1. A silk fibroin article comprising semi-crystalline silk fibroin, wherein the silk fibroin article has a glass transition temperature between about 40° C. to 120° C., wherein a flexural strength of the silk fibroin article is at least 5 MPa and density of the entire silk fibroin article is at least 1.20 g/cm3.
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