| CPC C07F 15/0033 (2013.01) [C07F 15/002 (2013.01); C07F 15/0086 (2013.01); H10K 85/342 (2023.02); H10K 85/346 (2023.02); H10K 85/348 (2023.02); H10K 50/11 (2023.02); H10K 85/40 (2023.02); H10K 85/622 (2023.02); H10K 85/654 (2023.02); H10K 85/6572 (2023.02); H10K 85/6576 (2023.02)] | 18 Claims |

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1. A compound comprising a first ligand LA of Formula I
![]() wherein Z1 to Z4 are each independently C or N;
two of Z1 to Z4 are N, and the remainder are C;
wherein ring A is Formula II
![]() wherein each RA and R4 independently represents mono substitution to a maximum possible number of substitutions, or no substitution;
wherein Z5 to Z8 are each independently C or N;
wherein R3 is a hydrogen or a substituent selected from the group consisting of deuterium, fluorine, alkyl, cycloalkyl, heteroalkyl, alkoxy, aryloxy, amino, silyl, aryl, and heteroaryl;
wherein each RA and R4 is independently a hydrogen or a substituent selected from the group consisting of deuterium, halogen, alkyl, cycloalkyl, heteroalkyl, heterocycloalkyl, arylalkyl, alkoxy, aryloxy, amino, silyl, alkenyl, cycloalkenyl, heteroalkenyl, alkynyl, aryl, heteroaryl, acyl, carboxylic acid, ether, ester, nitrile, isonitrile, sulfanyl, sulfinyl, sulfonyl, phosphino, and combinations thereof;
wherein any two substituents can be joined or fused together to form a ring;
wherein R3 and ring A do not have identical formulas;
wherein the ligand LA is complexed to a metal M;
wherein M is optionally coordinated to other ligands;
wherein the ligand LA is optionally linked with other ligands to comprise a tridentate, tetradentate, pentadentate, or hexadentate ligand; and
wherein if Z1 is N, the compound is homoleptic, or M is complexed to at least one substituted or unsubstituted acetylacetonate ligand.
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