| CPC H01M 4/505 (2013.01) [C01G 53/50 (2013.01); H01M 4/525 (2013.01); H01M 10/0525 (2013.01); H01M 10/0567 (2013.01); H01M 10/0568 (2013.01); H01M 10/0569 (2013.01); C01P 2006/40 (2013.01); H01M 2004/021 (2013.01); H01M 2004/028 (2013.01); H01M 2300/0037 (2013.01)] | 19 Claims |
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1. A lithium ion secondary battery comprising a battery core and an electrolyte, wherein:
the battery core comprises a negative electrode active material and a lithium-manganese-based positive electrode active material;
wherein the lithium-manganese-based positive electrode active material comprises first lithium-manganese-based positive electrode active material represented by chemical formula (1) and second lithium-manganese-based positive electrode active material represented by chemical formula (2),
Li1+xMnaNibM1−a−bO2−yAy Chemical formula (1)
in the chemical formula (1), −0.1≤x≤0.2, 0<a<1, 0≤b<1, 0<a+b<1, 0≤y<0.2, and M is one or more of Co, Fe, Cr, Ti, Zn, V, Al, Zr and Ce; A comprises one or more of S, N, F, Cl, Br and I;
Li1+zMncN2−cO4−dBd Chemical formula (2)
in the chemical formula (2), −0.1≤z≤0.2, 0<c≤2, 0≤d<1, and N comprises one or more of Ni, Fe, Cr, Ti, Zn, V, Al, Mg, Zr and Ce, and B comprises one or more of S, N, F, Cl, Br and I;
the electrolyte comprises a solvent, a lithium salt and an additive, and the additive comprises vinylene carbonate; and
wherein weight percentage q of the electrolyte based on a total weight of the positive electrode active material layer in the battery core is from 50 wt % to 70 wt %, weight percentage r of vinylene carbonate present in the electrolyte is from 0.01 wt % to 3.5 wt %, compaction density s of negative electrode active material layer in the battery core is from 1.3 g/cm3 to 1.65 g/cm3, and weight percentage p of manganese element present in the positive electrode active material is from 5 wt % to 50 wt %, and q, r, s, p satisfy formula (1):
![]() in the formula (1), the units of q, r, and p are wt %, and the unit of s is g/cm3.
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