| CPC H01L 21/0228 (2013.01) [C23C 16/45536 (2013.01); C23C 16/45544 (2013.01); C23C 16/52 (2013.01); H01J 37/32449 (2013.01); H01J 37/32724 (2013.01); H01J 37/32816 (2013.01); H01L 21/0217 (2013.01); H01L 21/02274 (2013.01); H01J 2237/332 (2013.01)] | 14 Claims |

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1. A method of manufacturing a semiconductor device, comprising
(A) forming a film containing a predetermined element and nitrogen on a substrate by performing a cycle a predetermined number of times,
wherein the cycle comprises:
(a) forming a first layer by supplying a source gas containing the predetermined element and a halogen element to the substrate heated to a first temperature in a process chamber;
(b) forming a second layer by modifying the first layer by supplying a first modification gas containing hydrogen free of nitrogen and exited by plasma to the substrate in the process chamber; and
(c) forming a third layer by modifying the second layer by supplying a second modification gas containing nitrogen and hydrogen and exited by plasma to the substrate in the process chamber, and
wherein a supply time TH of supplying the first modification gas in (b) is set to be longer than a supply time TN of supplying the second modification gas in (c).
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