| CPC H01L 21/76843 (2013.01) [C23C 16/34 (2013.01); C23C 16/45527 (2013.01); H01L 21/28556 (2013.01)] | 24 Claims |

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1. A method of forming a thin film comprising titanium nitride (TiN) by a cyclical vapor deposition process, the method comprising:
forming on a semiconductor substrate a TiN thin film by exposing the semiconductor substrate to one or more cyclical vapor deposition cycles each comprising an exposure to a Ti precursor at a Ti precursor flow rate and an exposure to a N precursor at a N precursor flow rate,
wherein the Ti precursor is exposed to the semiconductor substrate in the absence of any N precursor,
wherein a ratio of the N precursor flow rate to the Ti precursor flow rate (N/Ti flow ratio) exceeds 3, and
wherein the method forms the TiN thin film having a crystalline texture such that an X-ray spectrum of the TiN thin film has a ratio of a peak height or an intensity of an X-ray diffraction peak corresponding to a (111) crystal orientation of TiN to a peak height or an intensity of an X-ray diffraction peak corresponding to a (200) crystal orientation of TiN that exceeds 0.4.
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