| CPC H01M 10/0525 (2013.01) [H01M 4/131 (2013.01); H01M 4/134 (2013.01); H01M 4/623 (2013.01); H01M 2004/027 (2013.01); H01M 2004/028 (2013.01)] | 15 Claims |

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1. A lithium secondary battery comprising a positive electrode, a negative electrode, a separator, and an electrolyte,
wherein the positive electrode comprises a positive electrode active material layer comprising a positive electrode active material comprising an overlithiated manganese-based oxide represented by Formula 1 below, and
the negative electrode comprises a negative electrode active material layer comprising a silicon-based negative electrode active material,
LiaNibCocMndMeO2 [Formula 1]
wherein, 1<a, 0≤b≤0.5, 0≤c≤0.08, 0.5≤d<1.0, and 0≤e≤0.2, and M is at least one selected from the group consisting of Al, B, Co, W, Mg, V, Ti, Zn, Ga, In, Ru, Nb, Sn, Sr, and Zr,
wherein the positive electrode has an electrode density of 2.5 g/cc to 3.8 g/cc.
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