| CPC G02F 1/3617 (2013.01) [C07D 487/00 (2013.01); G02F 1/0018 (2013.01); G02F 1/3612 (2013.01)] | 7 Claims |

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1. A nonlinear optical chromophore of the general formula (I):
D-Π-A (I)
wherein D represents an organic electron-donating group; A represents an organic electron-accepting group having an electron affinity greater than the electron affinity of D; and Π represents a Π-bridge between the organic electron-accepting group and the organic electron-donating group; wherein the Π-bridge has the following formula (Πd):
![]() wherein Y represents: a sulfur linked aryl group; wherein each a and b independently represents an integer of 0 to 3; and z represents an integer of 1 to 3;
the nonlinear optical chromophore comprising one or more diamondoids, wherein one diamondoid of the one or more diamondoids is covalently bound to the organic electron-donating group.
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