| CPC H01M 4/366 (2013.01) [H01M 4/0428 (2013.01); H01M 4/386 (2013.01); H01M 4/58 (2013.01); H01M 4/626 (2013.01); H01M 10/0525 (2013.01); H01M 2004/021 (2013.01); H01M 2004/025 (2013.01); H01M 2004/027 (2013.01)] | 21 Claims |

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1. An anode for an energy storage device comprising:
a current collector comprising an electrically conductive layer;
a plurality of lithium storage filamentary structures in contact with the electrically conductive layer; and
a plurality of supplemental layers for each lithium storage filamentary structure of the plurality of lithium storage filamentary structures, wherein:
a first supplemental layer overlays at least a portion of the respective filamentary structure, the first supplemental layer comprising silicon nitride or a first metal compound, wherein the first metal compound comprises a metal oxide, a metal nitride, a metal oxynitride, a lithium-containing material, or a metalcone,
a second supplemental layer overlays at least a portion of the first supplemental layer, the second supplemental layer having a composition different from the first supplemental layer and comprising silicon nitride or a second metal compound, wherein the second metal compound comprises a metal oxide, a metal nitride, a metal oxynitride, a lithium-containing material, or a metalcone, and
a third supplemental layer overlaying at least a portion of the second supplemental layer, the third supplemental layer having a composition different from the second supplemental layer and comprising silicon nitride or a third metal compound.
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